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[Sweet and Sour] Vocaloid Unrequited Love Song Collection [Bittersweet]

There are many different forms of unrequited love.

Your heart might race nonstop with your first crush, or ache when you see the person you like talking to someone else.

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In this article, we’ve put together a selection of Vocaloid songs about unrequited love—perfect for those of you who are in love right now, or who want to remember how it felt back then.

As mentioned above, everyone has their own version of “unrequited love,” so we’ve picked out a wide variety of love songs!

You’re sure to find a track that perfectly matches your mood!

[Bittersweet] Vocaloid Unrequited Love Song Collection [Heartrending] (71–80)

Tohoku Kiritan’s Just-the-Two-of-Us☆ValentineSouth of South

Tohoku Kiritan’s Just-the-Two-of-Us☆Valentine (Full ver)
Tohoku Kiritan’s Just-the-Two-of-Us☆Valentine Minami no Minami

This is a Valentine’s song that sings of sweet, sweet love.

Released by Minami no Minami in February 2023, it’s included on the album “Minami no Zunpa CD.” The lyrics that depict pure feelings of love and the catchy melody are captivating.

The sparkling sound, the scenes of gifting a homemade cake, and spending a special time just for two let listeners feel the joy of being in love.

If you’re thinking about confessing but can’t take the first step, this might be the song that gently gives you a push.

If you want to feel your heart flutter, give it a listen!

KnockoutMerokuru

Knockout / Merokuru feat. Hatsune Miku
Knockout Merokuru

MeroKuru’s track “Knockout” charms with a poppy, catchy sound centered on the push-and-pull of romance.

It was released in August 2023 as an entry in VOCALOID Collection 2023 Summer (Rookie).

You think you’ll win if you can get the other person to say “I like you,” yet before you know it, you’ve said it yourself—those lovestruck feelings come through and make your heart skip a beat.

Coupled with Hatsune Miku’s cute vocals, just listening puts you in a romantic mood.

Perfect for Valentine’s Day or any time you want to feel a little special!

Thump-thump × Thump-thumpEon

[GUMI] Heart-Pounding × Heart-Pounding [Original Song HD]
Heart-Pounding × Heart-Pounding Eon

This is a very cute unrequited-love Vocaloid song whose lyrics express that floaty, giddy feeling you get when you’re in love.

One of the highlights is its sound, which is crafted to make you feel lighter as you listen.

Be sure to give it a careful listen.

[Bittersweet] Vocaloid Unrequited Love Song Collection [Heartrending] (81–90)

Pink Sugar CrushSakuramochi Luna

Pink Sugar Crush / Sakura Mochi Luna feat. Hatsune Miku
Pink Sugar Crush Sakura Mochi Luna

This work by Sakuramochi Luna is a track unveiled in March 2023 and included on the album “Mochi Town!” released in September.

The lyrics portray a protagonist who, while drowning in sweet temptation, struggles in pursuit of happiness, and Hatsune Miku’s transparent vocals further highlight those complex emotions.

It’s a song we especially recommend to anyone feeling the ache of unrequited love or the pain of a love that can’t come true.

This track may give you the chance to face the true feelings deep within your heart.

Fireworks in Your Colorfair-skinned

[GUMI] Kimi-iro Hanabi [Original PV]
Pale fireworks in your color

It’s a song that perfectly captures unrequited love—the feeling of “I need to tell you,” yet never quite getting the words out.

The guitar and bass are powerful, driving the melody forward.

But as the lyrics move like a reflection on the words left unsaid, what you feel is a deep poignancy.

It makes you think, “There are loves like this, and maybe that’s not such a bad thing.”

I'm sorry to you.Fei-P

Sorry to You (feat. Megpoid & Megurine Luka)
Sorry to you, Fay-P.

An original song by Fei-P that expresses a heartrending, poignant love through a light, buoyant melody.

Released in June 2009, this piece is notable for GUMI’s adorable vocals.

The lyrics depict the interplay between self-loathing and deep affection for the other person, conveying the frustration of feelings that can’t be put into words.

It’s recommended for anyone who relates to a single-minded unrequited love that becomes emotionally heavy because you care too much.

I believe the vocal range is comfortable for female singers.

squeak squeakhakame

Chiuchiu depicts unrequited love through a slightly unusual metaphor.

Created by Vocaloid producer Hakame as an entry for the 2023 Joke Song Posting Festival, its lyrics take the surprising subject of a lovesick mosquito.

The humor-filled writing makes it enjoyable to read on its own.

Every onomatopoeic phrase is catchy and approachable, and there’s a faintly bittersweet atmosphere that draws you in emotionally.

The music video, which personifies the mosquito, is also a must-see.