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[Sweet and Sour] Vocaloid Unrequited Love Song Collection [Bittersweet]

There are many different forms of unrequited love.

Your heart might race nonstop with your first crush, or ache when you see the person you like talking to someone else.

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In this article, we’ve put together a selection of Vocaloid songs about unrequited love—perfect for those of you who are in love right now, or who want to remember how it felt back then.

As mentioned above, everyone has their own version of “unrequited love,” so we’ve picked out a wide variety of love songs!

You’re sure to find a track that perfectly matches your mood!

[Bittersweet] Vocaloid Unrequited Love Song Collection [Heart-wrenching] (21–30)

Meltryo

When it comes to Hatsune Miku, this is the song everyone mentions!! It’s a famous track that always comes up in the conversation.

It sings about the bittersweet feelings of unrequited love.

You’re left with that fluttery, hazy excitement—did they end up together in the end or not? The song was created by ryo, the composer of the creative unit supercell.

CinderellaDECO*27

DECO*27 – Cinderella feat. Hatsune Miku
Cinderella DECO*27

When it comes to Vocaloid unrequited love songs overflowing with pure feelings for someone you like, “Cinderella” comes to mind.

Created in 2021 by DECO*27, a Vocaloid producer with many signature tracks, it resonates with a passionate sound that brilliantly crosses over electronica and band elements.

Many listeners will relate to the cute, girlish lyrics that depict a heart in love.

Also pay attention to Hatsune Miku’s pop vocal delivery that matches the song’s rhythmic tempo.

It’s an energetic number that wraps up the anxieties and loneliness of unrequited love.

Ambiguous Lust LoverDenpol-P

[flower] “Ambiguous Lust Lover” [Original]
Ambiguous Lewdness Lover by Denporu-P (Electric Love P)

Even though you have feelings for him and you’re putting yourself out there, he still won’t give you a clear answer! This is recommended for anyone who knows that kind of one-sided love.

Listen to this song and its straightforward lyrics will clear away the haze in your heart! Let’s blow away all those muddled feelings!

Repeat Onecat bug

[Kagamine Rin] Repeat One Grain [Original].mp4
Repeated single-grain cat bug

This is a recommended song for those suffering from painful unrequited love or those who want a good cry to feel refreshed.

The lyrics may verge on self-loathing, but anyone troubled by love will relate at least a little.

A song that brings to mind the phrase, “Love is just a passing fancy.”

about meChouchou-P

This is a track you’ll get hooked on for its cool vibe and English lyrics.

The words about being alone in a bedroom—knowing they won’t come, yet being unable to forget the person you love—are deeply moving.

Recommended for girls with a one-sided crush who want to feel a little more grown-up.

Izayoi MoonlightYūra

Izayoi Moonlight – Yuzuki Yukari
Izayoi Moonlight Yuura

It exudes a somewhat urban atmosphere and sings about the missed connections of adult romance.

“Izayoi Moonlight” is a song released in June 2021, created by Yuura.

Its refined piano sound stands out, giving the track a more stylish feel.

The string tones that enter during the interlude add a romantic touch, making it easy to picture the scenes the song portrays.

Recommended for those experiencing a mature love—one that requires you to wear even its bittersweetness with grace.

Happy SynthesizerEasy Pop

[Megurine Luka, GUMI] Happy Synthesizer [Original Song]
Happy Synthesizer Easy Pop

It’s a duet song by GUMI and Megurine Luka.

The poppy electronic sound and cute vocals naturally make your body sway as you listen.

It feels like it cheers on a tender crush, and it’s a song that makes you think, maybe I shouldn’t just hold back—maybe I should be honest about my feelings.